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Volume 15 Issue 4
Sep.  2013
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Study of ultrafast relaxation phenomena by a tunable laser induced transient grating

  • Received Date: 1990-06-01
    Accepted Date: 1990-12-26
  • The functional relationship between the diffraction efficiency τi(⊿ω)of a tunable-laser induced transient grating and the lifetime in ith energy level is derived from the theory of three-level rate equations and Maxwell equations.In this paper,the diffraction line shape τi(⊿ω)is analyzed and discussed.The experiment result of the longitudinal relaxation time T1 associated with the S0-S1 electronic transition of Malachite Green solution is also reported.
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    Trebino R,Barker C E,Siegman A E.Tunable-laser-induced gratings for the measurement of ultrafast phenomena.IEEE J Q E,1986;22(8):1413.
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    Fork R L,Cruz C H B,Becker P C et al.Compression of optical pulses to six femtoseconds by using cubic phase compensation.OPt Lett,1987;12(7):483-485.
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    Siegman A E.Proposed picosecond excited-state measurement method using a tunable-laser-induced grating.A P L,1977;30(1):21-23.
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    Sundström V,Gillbro T.Effects of solvent on TMP photophysics:Transition from no barrier to barrier cases,induced by solvent properties.J Chem Phys,1984,81(8):3463-3473.
    [5] 费浩生,张云,韩力et al.用喇曼增强非简并回波混频测量喇曼模的横向弛豫时间.物理学报,1989;38(12):2054.

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    Stavola M,Mourou G,Knox W.Picosecond time delay fluorzmetry using a jitter-free Streak camera.Opt Comm,1980;34(3):404.
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    Trebino R,Siegman A E.Subpicosecond relaxation study of malachite green using a three-laser frequency-domain technique.J Chem phys,1983;79(8):3621-3626.
    [8] 吕振国,符昌海,李庆行et al.共振混频过程的超快弛豫现象研究.激光技术,1990;14(5):10

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    沈阳化工大学材料科学与工程学院 沈阳 110142

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Study of ultrafast relaxation phenomena by a tunable laser induced transient grating

  • 1. Institute of Laser and Spectroscopy, Zhongshan University

Abstract: The functional relationship between the diffraction efficiency τi(⊿ω)of a tunable-laser induced transient grating and the lifetime in ith energy level is derived from the theory of three-level rate equations and Maxwell equations.In this paper,the diffraction line shape τi(⊿ω)is analyzed and discussed.The experiment result of the longitudinal relaxation time T1 associated with the S0-S1 electronic transition of Malachite Green solution is also reported.

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